A fresh look at 3D microwave ionization curves of hydrogen Rydberg atoms

A scheme for measurement of microwave (MW) electric field is proposed via multi-photon coherence in Rydberg atoms. It is based on the three-photon electromagnetically induced absorption (TPEIA) spectrum. In this process, the multi-photon produces a narrow absorption peak, which has a larger magnitude than the electromagnetically induced transparency (EIT) peak under the same conditions. The TPEIA peak is sensitive to MW fields, and can be used to measure MW electric field str...

We study the field-ionization threshold behavior when a Rydberg atom is ionized by a short single-cycle pulse field. Both hydrogen and sodium atoms are considered. The required threshold field amplitude is found to scale \emph{inversely} with the binding energy when the pulse duration becomes shorter than the classical Rydberg period, and, thus, more weakly bound electrons require larger fields for ionization. This threshold scaling behavior is confirmed by both 3D classical ...

The dynamics of Rydberg states of atomic hydrogen perturbed simultaneously by a static electric field and a resonant microwave field of elliptical polarization is analysed in the quantum perturbative limit of small amplitudes. For some configurations, the secular motion (i.e. evolution in time of the elliptical electronic trajectory) may be classically predominantly chaotic. By changing the orientation of the static field with respect to the polarization of the microwave fiel...

Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates, various types of static and dynamic disorder and on relaxation processes. However, two-dimensional spectra can be difficult to interpret without precise knowledge of how the signal components relate to microscopic Hamiltonian parameters and s...

Experiments have shown that the microwave ionization probability of a highly excited almost monodimensional hydrogen atom subjected to a microwave pulse sometimes grows in steps when the peak electric field of the pulse is increased. Classical pulsed simulations display the same steps, which have been traced to phase-space metamorphoses. Quantum numerical calculations again exhibit the same ionization steps. I show that the time-sequence of two level interactions, responsible...

Comparison of precision frequency measurements to quantum electrodynamics (QED) predictions for Rydberg states of hydrogen-like ions can yield information on values of fundamental constants and test theory. With the results of a calculation of a key QED contribution reported here, the uncertainty in the theory of the energy levels is reduced to a level where such a comparison can yield an improved value of the Rydberg constant.

Dynamical localization prevents driven atomic systems from fast fragmentation by hampering the excitation process. We present numerical simulations within a collinear model of microwave-driven helium Rydberg atoms and prove that dynamical localization survives the impact of electron-electron interaction, even for doubly excited states in the presence of fast autoionization. We conclude that the effect of electron-electron repulsion on localization can be described by an appro...

Microwave electric field sensing is of importance for a wide range of applications in areas of remote sensing, radar astronomy and communications. Over the past decade, Rydberg atoms, owing to their exaggerated response to microwave electric fields, plentiful optional energy levels and integratable preparation methods, have been used in ultra-sensitive, wide broadband, traceable, stealthy microwave electric field sensing. This review first introduces the basic concept of quan...

The results of a theoretical investigation of prompt many-body ionization are reported. Our calculations address an experiment that reported ionization in Rydberg gases for densities two orders of magnitude less than expected from ionization between pairs of atoms. The authors argued that the results were due to the simultaneous interaction between many atoms. We performed classical calculations for many interacting Rydberg atoms with the ions fixed in space and have found th...

We consider the dynamics of Rydberg states of the hydrogen atom driven by a microwave field of elliptical polarization, with a possible additional static electric field. We concentrate on the effect of a resonant weak field - whose frequency is close to the Kepler frequency of the electron around the nucleus - which essentially produces no ionization of the atom, but completely mixes the various states inside an hydrogenic manifold of fixed principal quantum number. For suffi...