March 5, 2009
Studies of random close packing of spheres have advanced our knowledge about the structure of systems such as liquids, glasses, emulsions, granular media, and amorphous solids. When these systems are confined their structural properties change. To understand these changes we study random close packing in finite-sized confined systems, in both two and three dimensions. Each packing consists of a 50-50 binary mixture with particle size ratio 1.4. The presence of confining walls significantly lowers the overall maximum area fraction (or volume fraction in three dimensions). A simple model is presented which quantifies the reduction in packing due to wall-induced structure. This wall-induced structure decays rapidly away from the wall, with characteristic length scales comparable to the small particle diameter.
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July 22, 2013
By means of numerical simulations, we study the influence of confinement on three-dimensional random close packed (RCP) granular materials subject to gravity. The effects of grain shape (spherical or polyhedral) and polydispersity on this dependence are investigated. In agreement with a simple geometrical model, the solid fraction is found to decrease linearly for increasing confinement no matter the grain shape. This decrease remains valid for bidisperse sphere packings alth...
December 10, 2012
We study numerically the influence of confinement on the solid fraction and on the structure of three-dimensional random close packed (RCP) granular materials subject to gravity. The effects of grain shape (spherical or polyhedral), material polydispersity and confining wall friction on this dependence are investigated. In agreement with a simple geometrical model, the solid fraction is found to decrease linearly for increasing confinement no matter the grain shape. Furthermo...
May 4, 2022
We present a theoretical prediction on random close packing factor \phi_RCP^b of binary granular packings based on the hard-sphere fluid theory. An unexplored regime is unravelled, where the packing fraction \phi_RCP^b is smaller than that of the mono-sized one \phi_RCP^m, i.e., the so-called loose jamming state. This is against our common perception that binary packings should always reach a denser packing than mono-sized packings at the jamming state. Numerical evidence fur...
February 24, 2014
Random packings of objects of a particular shape are ubiquitous in science and engineering. However, such jammed matter states have eluded any systematic theoretical treatment due to the strong positional and orientational correlations involved. In recent years progress on a fundamental description of jammed matter could be made by starting from a constant volume ensemble in the spirit of conventional statistical mechanics. Recent work has shown that this approach, first intr...
We apply a recent one-dimensional algorithm for predicting random close packing fractions of polydisperse hard spheres [Farr and Groot, J. Chem. Phys. 133, 244104 (2009)] to the case of lognormal distributions of sphere sizes and mixtures of such populations. We show that the results compare well to two much slower algorithms for directly simulating spheres in three dimensions, and show that the algorithm is fast enough to tackle inverse problems in particle packing: designin...
March 25, 2000
Despite its long history, there are many fundamental issues concerning random packings of spheres that remain elusive, including a precise definition of random close packing (RCP). We argue that the current picture of RCP cannot be made mathematically precise and support this conclusion via a molecular dynamics study of hard spheres using the Lubachevsky-Stillinger compression algorithm. We suggest that this impasse can be broken by introducing the new concept of a maximally ...
May 22, 2016
Maximally random jammed (MRJ) particle packings can be viewed as prototypical glasses in that they are maximally disordered while simultaneously being mechanically rigid. The prediction of the MRJ packing density phi, among other packing properties of frictionless particles, still poses many theoretical challenges, even for congruent spheres or disks. Using the geometric-structure approach, we derive for the first time a highly accurate formula for MRJ densities for a very wi...
August 17, 2022
We simulate a hard-sphere liquid in confined geometry where the separation of the two parallel, hard walls is smaller than two particle diameters. By systematically reducing the wall separation we analyze the behavior of structural and thermodynamic properties, such as inhomogeneous density profiles, structure factors, and compressibilities when approaching the two-dimensional limit. In agreement with asymptotic predictions, we find for quasi-two-dimensional fluids that the d...
January 30, 2012
Monodisperse circular disks have been collectively packed in confined geometries using a Monte Carlo method where the compaction is propelled by two- dimensional stochastic agitation. We have found that confinement (i.e., finite-size plus surface effects) determines the symmetry of the packed configurations together with the size evolution of the probability density of the packing fraction. For the particular case of small systems in square containers, the probability density...
June 6, 2010
We develop a model to describe the properties of random assemblies of polydisperse hard spheres. We show that the key features to describe the system are (i) the dependence between the free volume of a sphere and the various coordination numbers between the species, and (ii) the dependence of the coordination numbers with the concentration of species; quantities that are calculated analytically. The model predicts the density of random close packing and random loose packing o...