March 19, 2012
We explore the anisotropic nature of Feshbach resonances in the collision between ultracold magnetic submerged-shell dysprosium atoms, which can only occur due to couplings to rotating bound states. This is in contrast to well-studied alkali-metal atom collisions, where most Feshbach resonances are hyperfine induced and due to rotation-less bound states. Our novel first-principle coupled-channel calculation of the collisions between open-4f-shell spin-polarized bosonic dysprosium reveals a striking correlation between the anisotropy due to magnetic dipole-dipole and electrostatic interactions and the Feshbach spectrum as a function of an external magnetic field. Over a 20 mT magnetic field range we predict about a dozen Feshbach resonances and show that the resonance locations are exquisitely sensitive to the dysprosium isotope.
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October 14, 2014
This paper reviews current experimental and theoretical progress in the study of dipolar quantum gases of ground and meta-stable atoms with a large magnetic moment. We emphasize the anisotropic nature of Feshbach resonances due to coupling to fast-rotating resonant molecular states in ultracold s-wave collisions between magnetic atoms in external magnetic fields. The dramatic differences in the distribution of resonances of magnetic $^7$S$_3$ chromium and magnetic lanthanide ...
June 5, 2015
We report on the observation of weakly-bound dimers of bosonic Dysprosium with a strong universal s-wave halo character, associated with broad magnetic Feshbach resonances. These states surprisingly decouple from the chaotic backgound of narrow resonances, persisting across many such narrow resonances. In addition they show the highest reported magnetic moment $\mu\simeq20\,\mu_{\rm B}$ of any ultracold molecule. We analyze our findings using a coupled-channel theory taking i...
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We report the observation of resonance-like loss in the trap population of ultracold dysprosium as a function of magnetic field, which we attribute to anisotropy-induced Fano-Feshbach resonances arising from Dy's large magnetic dipole moment and nonzero electronic orbital angular momentum. We recorded these resonances for four different isotopes, three bosonic and one fermionic, over a field range of 0-6 G and show that the number of resonances changes significantly as a func...
March 28, 2018
We produce Bose-Einstein condensates of $^{162}$Dy atoms employing an innovative technique based on a resonator-enhanced optical trap that allows efficient loading from the magneto-optical trap and fast evaporation. We characterize the scattering properties of the ultracold atoms for magnetic fields between 6 and 30 G. In addition to the typical chaotic distribution of narrow Feshbach resonances in Lanthanides, we discover two rather isolated broad features at around 22 G and...
June 2, 2024
We report numerically exact quantum scattering calculations on magnetic Feshbach resonances in ultracold, strongly anisotropic atom-molecule [Rb($^2$S) + SrF($^2\Sigma^+$)] collisions based on state-of-the-art ab initio potential energy surfaces. We find broad resonances mediated by the intermolecular spin-exchange interaction, as well as narrow resonances due to the intramolecular spin-rotation interaction, which are unique to atom-molecule collisions. Remarkably, the densit...
October 24, 2003
We report a unique feature of magnetic field Feshbach resonances in which atoms collide with non-zero orbital angular momentum. P-wave ($l=1$) Feshbach resonances are split into two components depending on the magnitude of the resonant state's projection of orbital angular momentum onto the field axis. This splitting is due to the magnetic dipole-dipole interaction between the atoms and it offers a means to tune anisotropic interactions of an ultra-cold gas of atoms. A parame...
April 28, 2011
The nature of the interaction between ultracold atoms with a large orbital and spin angular momentum has attracted considerable attention. It was suggested that such interactions can lead to the realization of exotic states of highly correlated matter. Here, we report on a theoretical study of the competing anisotropic dispersion, magnetic dipole-dipole, and electric quadrupole-quadrupole forces between two dysprosium atoms. Each dysprosium atom has an orbital angular momentu...
December 1, 2009
Ultracold dysprosium gases, with a magnetic moment ten times that of alkali atoms and equal only to terbium as the most magnetic atom, are expected to exhibit a multitude of fascinating collisional dynamics and quantum dipolar phases, including quantum liquid crystal physics. We report the first laser cooling and trapping of half a billion Dy atoms using a repumper-free magneto-optical trap (MOT) and continuously loaded magnetic confinement, and we characterize the trap recyc...
February 17, 2015
We theoretically evaluate the feasibility to form magnetically-tunable Feshbach molecules in collisions between fermionic $^6$Li atoms and bosonic metastable $^{174}$Yb($^3$P$_2$) atoms. In contrast to the well-studied alkali-metal atom collisions, collisions with meta-stable atoms are highly anisotropic. Our first-principle coupled-channel calculation of these collisions reveals the existence of broad Feshbach resonances due to the combined effect of anisotropic-molecular an...
October 21, 2019
We have investigated Feshbach resonances in collisions of high-spin atoms such as Er and Dy with closed-shell atoms such as Sr and Yb, using coupled-channel scattering and bound-state calculations. We consider both low-anisotropy and high-anisotropy limits. In both regimes we find many resonances with a wide variety of widths. The wider resonances are suitable for tuning interatomic interactions, while some of the narrower resonances are highly suitable for magnetoassociation...