Coherence in magnetic quantum tunneling

We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and applying stationary approximation for excited doublets/singlets, we derive a key equation of motion for the quantum tunneling of magnetization process which is applicable in the whole temperature domain. From this equation, we find that in gene...

We generalize the Landau-Zener theory of coherent tunneling transitions by taking thermal relaxation into account. The evaluation of a new generalized master equation containing a dynamic tunneling rate that includes the interaction between the relevant system and its environment leads to an incoherent Zener transition probability with an exponent that is twice as large as the one of the coherent Zener probability in the limit T -> 0. We apply our results to molecular cluster...

It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of radiation in the terahertz range. Our analysis separates the time evolution into slow and fast components thereby obtaining an effective theory for the slow dynamics. This effective theory presents quenching of the tunnel effect. In particu...

The forerunners preceding the main tunneling signal of the wave created by a source with a sharp onset or by a quantum shutter, have been generally associated with over-the-barrier (non-tunneling) components. We demonstrate that, while this association is true for distances which are larger than the penetration lenght, for smaller distances the forerunner is dominated by under-the-barrier components. We find that its characteristic arrival time is inversely proportional to th...

We study macroscopic quantum coherence (MQC) in small ferrimagnets. Through semi-classical calculations we show that even a small uncompensated moment has a drastic effect on MQC. In particular, there is a rapid crossover to a regime where the MQC tunnel splitting is equal to that obtained for a ferromagnet, even though the system is still an antiferromagnet for all other aspects. We calculate this tunnel splitting via instanton methods and compare it with numerical evaluatio...

A new quantum approach is presented that can account for the description of small ferromagnetic particles magnetization tunneling. An estimate of the saturation value of an external applied magnetic field along the easy axis is obtained. An analytic expression for the tunneling factor in the absence of an external magnetic field is deduced from the present approach that also allows to obtain the crossover temperature characterizing the regime where tunneling is dominated by t...

Response to the Comment by Bellessa (arXiv:cond-mat/0006441).

We give a further step in the quantum mechanical description of engineered atomic spin structures by deriving a master equation of the Redfield type that governs the dynamics of the atomic spin density matrix. By generalizing this approach to charge-specific density matrices, we are able to describe magnetic transport quantities, such as the average inelastic current and the shot noise, accessible by tunneling spectroscopy. Our method suitably describes moderate lead-atom cou...

We report single-shot measurements of resistance versus time for thermally assisted spin-torque-driven switching in magnetic tunnel junctions. We achieve sufficient sensitivity to resolve the resistance signals leading up to switching, including the variations between individual switching events. Analyses of pre-switching thermal fluctuations allow detailed measurements of coherence times and variations in magnetization precession amplitude. We find that with a small in-plane...

In the regime of weak bath coupling and low temperature we demonstrate numerically for the spin-boson dynamics the equivalence between two widely used but seemingly different roads of approximation, namely the path integral approach and the Bloch-Redfield theory. The excellent agreement between these two methods is corroborated by a novel efficient analytical high-frequency approach: it well approximates the decay of quantum coherence via a series of damped coherent oscillati...