Thermal transport in a granular metal array

A user friendly scheme based on the quantum kinetic equation is developed for studying thermal transport phenomena in the presence of interactions and disorder. We demonstrate that this scheme is suitable for both a systematic perturbative calculation as well as a general analysis. We believe that we present an adequate alternative to the Kubo formula, which for the thermal transport is rather cumbersome.

We present a mesoscopic model for thermoelectric phenomena in terms of an interacting particle system, a lattice electron gas dynamics that is a suitable extension of the standard simple exclusion process. We concentrate on electronic heat and charge transport in different but connected metallic substances. The electrons hop between energy-cells located alongside the spatial extension of the metal wire. When changing energy level, the system exchanges energy with the environm...

We study thermoelectric properties of granular semiconductors with weak tunneling conductance between the grains, g_t < 1. We calculate the thermopower and figure of merit taking into account the shift of the chemical potential and the asymmetry of the density of states in the vicinity of the Fermi surface due to n- or p-type doping in the Efros-Shklovskii regime for temperatures less than the charging energy. We show that for weakly coupled semiconducting grains the figure o...

We study the thermoelectric effect of two-dimensional metals on a square lattice within semiclassical Boltzmann transport theory with particular focus on electron-electron scattering. We compute the electrical conductivity and the Seebeck coefficient as a function of band filling and temperature for generically chosen hopping parameters in a two-dimensional tight-binding model. The Boltzmann equation is solved numerically after computing the full collision integral, taking th...

We study charge transport in a granular array with high inter-grain conductances. We show that the system exhibits a Berezinskii-Kosterlitz-Thouless crossover from the high-temperature conducting state into a low-temperature insulating state. The crossover takes place at a critical temperature T_{BKT} \propto E_c exp{-g}, where E_c is the charging energy of a grain and g >> 1 is the dimensionless inter-grain conductance. A uniformly applied gate voltage drives the insulator i...

We prove that a diagrammatic evaluation of the Kubo formula for the electronic transport conductivity due the exchange of bosonic excitations, in the usual conserving ladder approximation, yields a result consistent with the Boltzmann equation. In particular, we show that an uncontrolled approximation that has been used to solve the integral equation for the vertex function is unnecessary. An exact solution of the integral equation yields the same asymptotic low-temperature b...

Metallic nanostructures (the nanofilms and nanowires) are widely used in electronic devices, and their thermal transport properties are crucial for heat dissipation. However, there are still gaps in understanding thermal transport in metallic nanostructures, especially regarding the size effect and validity of the Wiedemann-Franz law. In this work, we perform mode-by-mode first-principles calculations combining the Boltzmann transport equation to understand thermal transport ...

We present systematic theoretical results on thermoelectric effects in semimetals based on the variational method of the linearized Boltzmann equation. Inelastic electron-hole scattering is known to play an important role in the unusual transport of semimetals, including the broad $T^2$ temperature dependence of the electrical resistivity and the strong violation of the Wiedemann-Franz law. By treating the inelastic electron-hole scattering more precisely beyond the relaxatio...

We study thermal conductivity in the disordered two-dimensional electron liquid in the presence of long-range Coulomb interactions. We describe a microscopic analysis of the problem using as a starting point the partition function defined on the Keldysh contour. We extend the Renormalization Group (RG) analysis developed for thermal transport in the disordered Fermi liquid, and include scattering processes induced by the long-range Coulomb interaction in the sub-temperature e...

A fully predictive Kinetic Collective Model using first principles phonon spectra and relaxation times is presented. Thermal conductivity values obtained for Si, Ge, C (diamond) and GaAs in a wide range of sizes and temperatures have good agreement with experimental data without the use of any fitting parameter. This validation of the model open the door to discuss how the precise combination of kinetic and collective contributions to heat transport could provide a useful fra...