Electronic Theory for the Nonlinear Magneto-Optical Response of Transition-Metals at Surfaces and Interfaces: Dependence of the Kerr-Rotation on Polarization and on the Magnetic Easy Axis

In conventional Kerr- and Faraday microscopy the sample is illuminated with plane-polarised light and a magnetic domain contrast is generated by an analyser making use of the Kerr- or Faraday rotation. In this paper we demonstrate possibilities of analyser-free magneto-optical microscopy based on magnetisation-dependent intensity modulations of the light: (i) The transverse Kerr effect can be applied for in-plane magnetised material, demonstrated for an FeSi sheet. (ii) Illum...

Ultrafast magnetization dynamics in metallic heterostructures consists of a combination of local demagnetization in the ferromagnetic constituent and spin-dependent transport contributions within and in between the constituents. Separation of these local and non-local contributions is essential to obtain microscopic understanding and for potential applications of the underlying microscopic processes. By comparing the ultrafast changes of the polarization rotation and elliptic...

Co$_3$O$_4$, ZnFe$_2$O$_4$, CoFe$_2$O$_4$, ZnCo$_2$O$_4$, and Fe$_3$O$_4$ thin films were fabricated by pulsed laser deposition at high and low temperatures resulting in crystalline single-phase normal, inverse, as well as disordered spinel oxide thin films with smooth surface morphology. The dielectric function, determined by spectroscopic ellipsometry in a wide spectral range from 0.5 eV to 8.5 eV, is compared with the magneto-optical response of the dielectric tensor, inve...

A magneto-optically active thin film of Rb$_{j}$Co$_{k}$[Fe(CN)$_{6}$]$_{l}$ $\cdot$$n$H$_{2}$O has been prepared using a sequential assembly method. Upon irradiation with light and at 5 K, the net magnetization of the film increased when the surface of the film was oriented parallel to the external magnetic field of 0.1 T. However, when the surface of the film was perpendicular to the field, the net magnetization \emph{decreased} upon irradiation. The presence of dipolar fie...

We describe the phenomenon of optical activity of noncentrosymmetric metals in their normal and superconducting states. The found conductivity tensor contains the linear in wave vector off diagonal part responsible for the natural optical activity. Its value is expressed through the ratio of light frequency to the band splitting due to the spin-orbit interaction. The Kerr rotation of polarization of light reflected from the metal surface is calculated. In the additional fil...

Based on nonlinear optics, we develop a band theory to elucidate how light could manipulate magnetization, which is rooted by the quantum geometric structure and topological nature of electronic wavefunctions. Their existence are determined by the light polarization and specific material symmetry, based on the magnetic group theory. In general, both circularly and linearly polarized light could exert an effective magnetic field and torque effect, to reorient the magnetization...

We have performed ab initio studies to elucidate the unusual magnetic behavior recently observed in epitaxial Co films upon absorption of submonolayers of Cu and other materials. We find that a submonolayer amount of Cu on a stepped Co/Cu (100) film changes dramatically the electronic and magnetic structure of the system. The effect is mainly due to hybridization of Co and Cu $d$-electrons when copper forms a ``wire'' next to a Co step at the surface. As a result, a non-colli...

Magneto-optical Kerr effect, normally found in magnetic materials with nonzero magnetization such as ferromagnets and ferrimagnets, has been known for more than a century. Here, using first-principles density functional theory, we demonstrate large magneto-optical Kerr effect in high temperature noncollinear antiferromagnets Mn$_{3}X$ ($X$ = Rh, Ir, or Pt), in contrast to usual wisdom. The calculated Kerr rotation angles are large, being comparable to that of transition metal...

We report on the optical characterization of non-magnetic metal/ferromagnetic (Co$_{20}$Fe$_{60}$B$_{20}$)/MgO heterostructures and interfaces by using mid infrared spectroscopic ellipsometry at room temperature. We extracted for the mid-infrared range the dielectric function of Co$_{20}$Fe$_{60}$B$_{20}$, that is lacking in literature, from a multisample analysis. From the optical modelling of the heterostructures we detected and determined the dielectric tensor properties o...

An alternate method of measuring anisotropy fields in thin film ferromagnets is demonstrated. The method relies on the magnetic susceptibility in a small a.c. magnetic field, measured \txtit{in situ} using the magneto-optic Kerr effect (MOKE), and will be useful in situations where more specialized apparatus are not available, or constraints discourage the use of a large, static magnetic field. The method is demonstrated for Co/W(110) films, where it yields anisotropy fields ...