June 3, 1999
The cold(neutronless) fission of $^{252}$Cf is studied in the frame of a molecular model in which the scission configuration is described by two aligned fragments interacting by means of Coulomb (+ nuclear) forces. The study is carried out for different distances between the fragments tips and excitation energies. For a given deformation, the fragment's total energy is computed via the constrained Hartree-Fock + BCS formalism. The total excitation energy present in the fragments is supposed to contribute only to the fragments deformation and the asymptotic value of the kinetic energy is equated to the inter-fragment potential at scission. These two constraints yield not more than one or two fission channels for a fixed tip distance and excitation energy. Discarding those fission channels corresponding to a disequilibrated sharing of the excitation energy between the two fragments, we were able to establish the most likely scission configurations for a specified excitation energy.
Similar papers 1
October 30, 2000
The recent advent of experimental techniques in which the dynamical characteristics of fission fragments are determined more accurately, prompted us to investigate the angular momentum acquired by fragments in a model which describes the cold(neutronless) fission of $^{252}$Cf as the decay of a giant nuclear molecule. The molecular configuration is a consequence of the interplay between the attractive nuclear part and the repulsive Coulomb+nuclear forces. The basic ideea of t...
July 20, 2009
We investigate the cold fission of 252Cf within the two center shell model to compute the potential energy surface. The fission yields are estimated by using the semiclassical penetration approach. It turns out that the inner cold valley of the total potential energy is strongly connected with Z=50 magic number. The agreement with experimental values is very much improved only by considering mass and charge asymmetry degrees of freedom. Thus, indeed cold fission of 252Cf is a...
March 26, 1998
We predict a molecular vibrational state in the cold binary fission of $^{252}$Cf using a simple decay cluster model. The Hamiltonian of two even-even fragments in the pole-pole configuration is built in the same fashion as that for the dinuclear molecule formed in heavy-ions collisions. The interaction between the two fragments is described by the double-folding M3Y potential. The spectrum of the butterfly vibrations is derived and its dependence on fragments deformation and...
October 30, 2000
Based on a recent experimental finding which may suggest the existence of a tri-nuclear molecular structure before the cold ternary fragmentation of $^{252}$Cf takes place, we solved the eigenvalue problem of a certain class of vibrations which are very likely to occur in these molecules. These oscillations are the result of the joined action of rotations of the heavier fragments and the transversal vibrations of the lighter spherical cluster with respect to the fission axis....
January 12, 2015
Upon increasing significantly the nuclear elongation, the beta-decay energy grows. This paper investigates within a simple yet partly microscopic approach, the transition rate of the beta decay of the 252Cf nucleus on the way to scission from the exit point for a spontaneous fission process. A rather crude classical approximation is made for the corresponding damped collective motion assumed to be one dimensional. Given these assumptions, we only aim in this paper at providin...
December 17, 2013
Although the overall time-scale for nuclear fission is long, suggesting a slow process, rapid shape evolution occurs in its later stages near scission. Theoretical prediction of the fission fragments and their characteristics are often based on the assumption that the internal degrees of freedom are equilibrated along the fission path. However, this adiabatic approximation may break down near scission. This is studied for the symmetric fission of $^{258,264}$Fm. The non-adiab...
August 25, 2024
Current work discusses methods for estimating the moments of inertia of fission fragments for spontaneous fission of the isotope Cf-252, in particular, two main approaches are mentioned: statistical and microscopic. In addition, the methods of the classical and superfluid approaches to the calculation of the moments of inertia are discussed, as well as their application to different models of nuclei. Within this framework, the influence of different oscillation modes and nucl...
August 9, 2021
We present the first fully unrestricted microscopic calculations of the primary fission fragment intrinsic spins and of the fission fragments' relative orbital angular momentum for $^{236}$U$^*$, $^{240}$Pu$^*$, and $^{252}$Cf using the time-dependent density functional theory framework. Within this microscopic approach, free of restrictions and unchecked assumptions and which incorporates the relevant physical observables for describing fission, we evaluate the triple distri...
August 1, 1998
We compute the final kinetic energies of the fragments emitted in the light charged particle accompanied cold fission of $^{252}$Cf taking into account the ground state quadrupole deformation and the finite-size effects of the fragments and integrating the equations of motion for a three-body system subjected only to Coulomb forces. The initial conditions for the trajectory calculations were derived in the frame of a deformed cluster model which includes also the effect due t...
October 9, 2009
Fission-fragment properties have been calculated for thermal neutron-induced fission on a $^{239}\textrm{Pu}$ target, using constrained Hartree-Fock-Bogoliubov calculations with a finite-range effective interaction. A quantitative criterion based on the interaction energy between the nascent fragments is introduced to define the scission configurations. The validity of this criterion is benchmarked against experimental measurements of the kinetic energies and of multiplicitie...