Lanczos Study of the S=1/2 Frustrated Square-Lattice Antiferromagnet in a Magnetic Field

We present a model compound with a spin-1/2 frustrated square lattice, in which three ferromagnetic (F) interactions and one antiferromagnetic (AF) compet. Considering the effective spin-1 formed by the dominant F dimer, this square lattice can be mapped to a spin-1 spatially anisotropic triangular lattice. The magnetization curve exhibits gapped behavior indicative of a dominant one-dimensional (1D) AF correlation. In the field-induced gapless phase, the specific heat and ma...

We present results from our analysis of the finite-temperature properties of the spin 1/2 $J_{1}$-$J_{2}$ Heisenberg model on a square lattice. The analysis is based on the exact diagonalization of small clusters with 16 and 20 sites utilizing the finite-temperature Lanczos method. In particular, we focus on the temperature dependence of the third-order magnetic susceptibility as a method to resolve the ambiguity of exchange constants. We discuss the entire range of the frust...

Motivated by the intriguing report, in some frustrated quantum antiferromagnets, of magnetization plateaus whose simple collinear structure is {\it not} stabilized by an external magnetic field in the classical limit, we develop a semiclassical method to estimate the zero-point energy of collinear configurations even when they do not correspond to a local minimum of the classical energy. For the spin-1/2 frustrated square-lattice antiferromagnet, this approach leads to the st...

We overview physical effects of exchange frustration and quantum spin fluctuations in (quasi-) two dimensional (2D) quantum magnets ($S=1/2$) with square, rectangular and triangular structure. Our discussion is based on the $J_1$-$J_2$ type frustrated exchange model and its generalizations. These models are closely related and allow to tune between different phases, magnetically ordered as well as more exotic nonmagnetic quantum phases by changing only one or two control para...

For the paradigmatic frustrated spin-half Heisenberg antiferromagnet on the kagome lattice we performed large-scale numerical investigation of thermodynamic functions by means of the finite-temperature Lanczos method for system sizes of up to N=42. We present the dependence of magnetization as well as specific heat on temperature and external field and show in particular that a finite-size scaling of specific heat supports the appearance of a low-temperature shoulder below th...

We develop a general framework, which combines exact diagonalization in small clusters with a density matrix variational principle, to study frustrated magnets at finite temperature. This thermodynamic hierarchical mean-field technique is used to determine the phase diagram and magnetization process of the three-dimensional spin-1/2 $J_1$-$J_2$ antiferromagnet on a stacked square lattice. Its non-magnetic phase exhibits a thermal crossover from a quantum to a classical parama...

We present a unified approach to the problem of degeneracy lifting in geometrically frustrated magnets with and without an external field. The method treats fluctuations around a classical spin configuration in terms of a real-space perturbation expansion. We calculate two lowest-order contributions for the Heisenberg spin Hamiltonian and use them to study the magnetization processes of spin-$S$ triangular and kagom\'e antiferromagnets.

In this work a site diluted antiferromagntic Ising model in the FCC lattice is studied by Monte Carlo simulation. At low temperatures, we find that as the external field is increased the transition from the antiferromagnetic phase to the superantiferromagnetic one occurs through an intermediate phase which is not present in the undiluted system. This new phase ordering has three distinct values for the sublattice magnetizations corresponding to one of the phases found in a re...

Using an exact diagonalization treatment of Ising and Heisenberg model Hamiltonians, we study field-induced phase transition for two-dimensional antiferromagnets. For the system of Ising antiferromagnet the predicted field-induced phase transition is of first order, while for the system of Heisenberg antiferromagnet it is the second-order transition. We find from the exact diagonalization calculations that the second-order phase transition (metamagnetism) occurs through a spi...

We discuss the ground state and the low-lying excitations of the spin-half Heisenberg antiferromagnet on the two-dimensional square-kagome lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite non-trivial degeneracy of the classical ground state as it is known also for the Heisenberg antiferromagnet on the kagome and on the star lattice. The quantum ground state of the spin-half system is a quantum paramagnet likely with a finit...