Spin-Glass State in $\rm CuGa_2O_4$

Muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagom\'{e} system (Cu$_x$Zn$_{1-x}$)$_{3}$V$_{2}$O$_7$(OH)$_{2}$ 2H$_2$O. In the pure $x=1$ system we found a slowing down of Cu spin fluctuations with decreasing temperature towards $T \sim 1$ K, followed by slow and nearly temperature-independent spin fluctuations persisting down to $T$ = 50 mK, indicative of quantum fluctuations. No indication of sta...

Muon spin rotation measurements supported by magnetization experiments have been carried out in a stoichiometric high-$T_c$ parent compound La$_2$CuO$_4$ in %the a temperature range from 2~K to 340~K and in transverse magnetic fields up to 5~T. Along with the antiferromagnetic local field, muon spin rotation spectra indicate presence of an additional source of magnetic field on the muon. The characteristic splitting of about 45~G coming from this additional magnetic field is ...

Within the wide class of disordered materials, spin glasses occupy a special place because of their conceptually simple definition of randomly interacting spins. Their modelling has triggered spectacular developments of out-of-equilibrium statistical physics, as well analytically as numerically, opening the way to a new vision of glasses in general. "Real" spin glasses are disordered magnetic materials which can be very diverse from the chemist's point of view, but all share ...

Tetragonal distorted spinel of CuMn2-xTixO4 (x = 0, 0.25 and 0.50) was prepared by solid state reaction method followed by neutron diffraction, FTIR spectroscopy, dielectric spectroscopy and magnetization measurements. The neutron diffraction and FTIR spectroscopy provide the information regarding phase formation. But, the magnetic susceptibility clearly shows the ferri-magnetic order below 76K associated with meta-magnetic state which turns to spin-glass behaviour upon Ti-su...

Experiments on the temperature and time dependence of the response function and the field cooled magnetisation of a Cu(Mn) spin glass at temperatures below the zero field spin glass temperature are used to explore the non-equilibrium nature of the underlying spin configuration. The results imply that a certain spin configuration is imprinted on the system as the temperature is decreased at a constant cooling rate. The cooling rate governs the magnitude of the FC magnetisation...

We have investigated the magnetic properties of CuNCN, the first nitrogen-based analogue of cupric oxide, CuO. Our muon spin relaxation, nuclear magnetic resonance and electron spin resonance studies reveal that classical magnetic ordering is absent down to lowest temperatures. However, large enhancement of spin correlations and unexpected inhomogeneous magnetism have been observed below 80 K. We attribute this to a peculiar fragility of the electronic state against weak pert...

We demonstrate via a muon spin rotation experiment that the electronic ground state of the iridium spinel compound, CuIr$_2$S$_4$, is not the presumed spin-singlet state but a novel paramagnetic state, showing a quasistatic spin glass-like magnetism below ~100 K. Considering the earlier indication that IrS$_6$ octahedra exhibit dimerization associated with the metal-to-insulator transition below 230 K, the present result suggests that a strong spin-orbit interaction may be pl...

Magnetic susceptibility and muon spin relaxation (muSR) experiments have been carried out on the quasi-2D triangular-lattice spin S = 2 antiferromagnet FeGa2S4. The muSR data indicate a sharp onset of a frozen or nearly-frozen spin state at T* = 31(2) K, twice the spin-glass-like freezing temperature T_f = 16(1) K. The susceptibility becomes field dependent below T*, but no sharp anomaly is observed in any bulk property. A similar transition is observed in muSR data from the ...

We have performed muon spin relaxation and susceptibility measurements of CaV_4O_9 and CaV_2O_5, systems in which spin gap-like behavior has been found. We observe spin freezing in the two compounds below 12K and 50K, respectively. Our results indicate the possibility that a substantial fraction of the of the vanadium magnetic moment is not in a spin singlet sate at low temperatures in either material.

We carried out AC magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ~1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type ground state, i.e. without broken symmetries or frozen moments. However, the AC susceptibility revealed a dilute-spin-glass like transition below ~ 1 K. Antiferromagnetically coupled Mo5+ 4d1 electrons in triply degenerate t2g orbitals are i...