Pump-probe differencing technique for cavity-enhanced, noise-canceling saturation laser spectroscopy

We report a simple technique for stabilization of a laser frequency at the wings of an atomic resonance. The reference signal used for stabilization issues from interference effects obtained in a low-quality cavity filled with a resonant atomic vapour. For a frequency detuned at 2.6 GHz from the $^{133}$Cs D$_2$ 6S$_{1/2}$ F=4 to 6P$_{3/2}$ F'= 5 transition, the fractional frequency Allan deviation is $10^{-8}$ for averaging times of 300 s, corresponding to a frequency deviat...

An experimental method is developed for the robust frequency stabilization using a high-finesse cavity when the laser exhibits large intermittent frequency jumps. This is accomplished by applying an additional slow feedback signal from Doppler-free fluorescence spectroscopy in an atomic beam with increased frequency locking range. As a result, a stable and narrow-linewidth 556 nm laser maintains the frequency lock status for more than a week, and contributes to more accurate ...

We report on the frequency locking of a frequency doubled Nd:YAG laser to a 45 000 finesse, 87-cm-long, Fabry-Perot cavity using a modified form of the Pound-Drever-Hall technique. Necessary signals, such as light phase modulation and frequency correction feedback, are fed direcly to the infrared pump laser. This is sufficient to achieve a stable locking of the 532 nm visible beam to the cavity, also showing that the doubling process does not degrade laser performances.

We propose and demonstrate a scheme to enable Doppler compensation within optical cavities for atom interferometry at significantly increased mode diameters. This has the potential to overcome the primary limitations in cavity enhancement for atom interferometry, circumventing the cavity linewidth limit and enabling mode filtering, power enhancement, and a large beam diameter simultaneously. This approach combines a magnified linear cavity with an intracavity Pockels cell. Th...

A spectrometer for ultra high-resolution spectroscopy of molecular iodine at wave length 501.7 nm, near the dissociation limit is described. Line shapes about 30 kHz wide (HWHM) were obtained using saturation spectroscopy in a pumped cell. The frequency of an Ar+ laser was locked to a hyperfine component of the R(26)62-0 transition and the first absolute frequency measurement of this line is reported.

We present high-resolution spectroscopy of Iodine vapour that is loaded and trapped within the core of a hollow-core photonic crystal fibre (HC-PCF). We compare the observed spectroscopic features to those seen in a conventional iodine cell and show that the saturation characteristics differ significantly. Despite the confined geometry it was still possible to obtain sub-Doppler features with a spectral width of ~6 MHz with very high contrast. We provide a simple theory which...

We have shown earlier that hyperfine spectroscopy in a vapor cell using co-propagating pump-probe beams has many advantages over the usual technique of saturated-absorption spectroscopy using counter-propagating beams. The main advantages are the absence of crossover resonances, the appearance of the signal on a flat (Doppler-free) background, and the higher signal-to-noise ratio of the primary peaks. Interaction with non-zero-velocity atoms causes additional peaks, but only ...

We propose a novel method that uses the oscillation of an atomic excited wave packet observed through a pump-probe technique to accurately determine the zero time delay between a pair of ultrashort laser pulses. This physically-based approach provides an easy fix for the intractable problem of synchronizing two different femtosecond laser pulses in a practical experimental environment, especially where an in situ time zero measurement with high accuracy is required.

High finesse Fabry-Perot(FP) cavity is a very important frequency reference for laser stabiliza- tion, and is widely used for applications such as precision measurement, laser cooling of ions or molecules. But the non-linear response of the piezoelectric ceramic transducer (PZT) in the FP cav- ity limits the performance of the laser stabilization. Measuring and controlling such non-linearity are important. Here we report an in-situ, optical method to characterize this non-lin...

State-of-the-art Doppler experiments require wavelength calibration with precision at the cm/s level. A low-finesse Fabry-Perot interferometer (FPI) can provide a wavelength comb with a very large bandwidth as required for astronomical experiments, but unavoidable spectral drifts are difficult to control. Instead of actively controlling the FPI cavity, we propose to passively stabilize the interferometer and track the time-dependent cavity length drift externally. A dual-fine...