Pump-probe differencing technique for cavity-enhanced, noise-canceling saturation laser spectroscopy

We present a new method of laser frequency locking in which the feedback signal is directly proportional to the detuning from an atomic transition, even at detunings many times the natural linewidth of the transition. Our method is a form of sub-Doppler polarization spectroscopy, based on measuring two Stokes parameters ($I_2$ and $I_3$) of light transmitted through a vapor cell. This extends the linear capture range of the lock loop by up to an order of magnitude and provide...

Vapour cell spectroscopy is an essential technique in many fields; in particular, nearly all atom and ion trapping experiments rely on simultaneous spectroscopy of two atomic transitions, traditionally employing separate apparatus for each transition. Here, we demonstrate simultaneous spectroscopy on two atomic transitions using spatially-overlapped beams from two independent lasers, within a single spectroscopic apparatus. We show that, in addition to aiding compactness, thi...

We stabilized the frequencies of two independent Nd:YAG lasers to two adjacent longitudinal modes of a high-finesse Fabry-P\'erot resonator and obtained a beat frequency instability of 6.3 mHz at an integration time of 40 s. Referred to a single laser, this is $1.6\times10^{-17}$ relative to the laser frequency, and $1.3\times10^{-6}$ relative to the full width at half maximum of the cavity resonance. The amplitude spectrum of the beat signal had a FWHM of 7.8 mHz. This stabl...

Avoiding laser frequency drifts is a key issue in many atomic physics experiments. Several techniques have been developed to lock the laser frequency using sub-Doppler dispersive atomic lineshapes as error signals in a feedback loop. We propose here a two-beam technique that uses non-linear properties of an atomic vapor around sharp resonances to produce sub-Doppler dispersive-like lineshapes that can be used as error signals. Our simple and robust technique has the advantage...

We propose a measurement of laser-induced vacuum birefringence through the use of pulsed lasers coupled to femtosecond optical enhancement cavities. This measurement technique features cavity-enhanced pump and probe pulses, as well as an independent control pulse. The control pulse allows for a differential measurement where the final signal is obtained using high-frequency lock-in detection, greatly mitigating time-dependent cavity birefringence as an important and possibly ...

Light from a Tm,Ho:YLF laser operating at 2051 nm is frequency doubled then coupled into a high Fabry-Perot cavity with manufacturer quoted finesse in excess of 300,000. The frequency of the laser is stabilized using the Pound-Drever-Hall (PDH) method. A two channel feedback circuit allows for laser frequency stabilization with a bandwidth of 2 MHz. This laser system has been used to drive the 6S1/2 to 5D3/2 transition in 138Ba+, where a 2 ms laser-ion coherence times has bee...

The optical manipulation of Ba$^{+}$ ions is mainly performed by a 493 nm laser for the S$_{1/2}$-P$_{1/2}$ transition and a 650 nm laser for the P$_{1/2}$-D$_{3/2}$ transition. Since the branching ratio between the 493 nm and 650 nm transitions of a single Ba$^{+}$ ion is comparable, stabilization systems of both lasers are equally important for Doppler cooling, sub-Doppler cooling, optical pumping and state detection. The stabilization system of a 493 nm laser to an absolut...

We measured the transition frequencies of the hyperfine components in the four lines (P(34) 39-0, R(36) 39-0, P(33) 39-0, and R(35) 39-0) of the B-X transitions of molecular iodine at 520.2 nm. The 520.2 nm laser was generated by wavelength-converting the output of a 1560.6 nm external-cavity diode laser using a dual-pitch periodically poled lithium niobate (PPLN) waveguide. The frequencies were measured by counting the heterodyne beats between the laser stabilized at the fre...

Many precision laser applications require active frequency stabilization. However, such stabilization loops operate by pushing noise to frequencies outside their bandwidth, leading to large "servo bumps" that can have deleterious effects for certain applications. The prevailing approach to filtering this noise is to pass the laser through a high finesse optical cavity, which places constraints on the system design. Here, we propose and demonstrate a different approach where a...

We investigate 13 hyperfine structures of transition lines of 127I2 near 554 nm, namely, the R(50) 22-0, P(46) 22-0, P(121) 24-0, P(69) 25-1, R(146) 25-0, R(147) 28-1, P(160) 26-0, P(102) 26-1, R(96) 23-0, R(49) 22-0, P(45) 22-0, P(92) 23-0, and R(72) 25-1 transitions, and measure their absolute frequencies with an optical frequency comb. A 369 nm frequency-tripled laser is frequency stabilized by locking the 554 nm harmonic-frequency laser to the R(146) 25-0 a15 line of 127I...