Enhancement and Inhibition of Stimulated Processes in a Negative Index Cavity

We demonstrate second and third harmonic generation from a GaP substrate 500{\mu}m thick. The second harmonic field is tuned at the absorption resonance at 335nm, and the third harmonic signal is tuned at 223nm, in a range where the dielectric function is negative. These results show that a phase locking mechanism that triggers transparency at the harmonic wavelengths persists regardless of the dispersive properties of the medium, and that the fields propagate hundreds of mic...

Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher harmonic conversion efficiencies per unit volume than those attainable in bulk materials. Here we demonstrate efficient second-harmonic generation (SHG) in a serrated nanogap plasmonic geometry that generates steep electric field gradients on...

The plasmon-enhanced second harmonic generation in the subwavelength neutral metal cubic nanoparticles is calculated for the first time in the hydrodynamic and cold plasma approximations. The theory is developed that takes into account all singularities of the electromagnetic field at the cubic nanoparticle surface. The results are compared to the linear case for the nanocube and to those for a spherical nanoparticle. In the latter case, they demonstrate very strong enhanceme...

Intrinsic to the process of high-order harmonic generation is the creation of plasma and the resulting spatiotemporal distortions of the driving laser pulse. Inside a high finesse cavity where the driver pulse and gas medium are reused, this can lead to optical bistability of the cavity-plasma system, accumulated self-phase modulation of the intracavity pulse, and coupling to higher order cavity modes. We present an experimental and theoretical study of these effects and disc...

We demonstrate unexpectedly strong second harmonic generation (SHG) in Argon gas by use of spatiotemporally focused (SF) femtosecond laser pulses. The resulting SHG by the SF scheme at a 75 cm distance shows a significantly enhanced efficiency than that achieved with conventional focusing scheme, which offers a new promising possibility for standoff applications. Our theoretical calculations reasonably reproduce the experimental observations, which indicate that the observed ...

We show, that engineering the cavity aspect ratio of AlGaAs micropillar resonator allows for the two order of magnitude increase in the efficiency of second harmonic generation at telecom wavelengths.

We demonstrate the simultaneous generation of second and third harmonic signals from a telecom wavelength pump in a gallium phosphide (GaP) microdisk. Using analysis of the power scaling of both the second and third harmonic outputs and calculations of nonlinear cavity mode coupling factors, we study contributions to the third harmonic signal from direct and cascaded sum frequency generation processes. We find that despite the relatively high material absorption in gallium ph...

We suggest a novel approach for generating second-harmonic radiation in subwavelength graphene waveguides. We demonstrate that quadratic phase matching between the plasmonic guided modes of different symmetries can be achieved in a planar double-layer geometry when conductivity of one of the layers becomes spatially modulated. We predict theoretically that, owing to graphene nonlocal conductivity, the second-order nonlinear processes can be actualized for interacting plasmoni...

A novel method for converting an array of out-of-phase lasers into one of in-phase lasers that can be tightly focused is presented. The method exploits second harmonic generation and can be adapted for different laser arrays geometries. Experimental and calculated results, presented for negatively coupled lasers formed in a square, honeycomb, and triangular geometries are in good agreement.

Plasmonic resonances in metallic nanostructures have been shown to drastically enhance local electromagnetic fields, and thereby increase the efficiency of nonlinear optical phenomena, such as second harmonic generation (SHG). While it has been experimentally observed that enhanced fields can significantly boost SHG, to date it proved difficult to probe electrical and magnetic resonances in one and the same nanostructure. This however is necessary to directly compare relative...