ID: cond-mat/0409178

Multi-Triplet Magnons in SrCu$_2$(BO$_3$)$_2$ Studied by Thermal Conductivity Measurements in Magnetic Fields

September 8, 2004

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Specific Heat of the S=1/2 Two-Dimensional Shastry-Sutherland Antiferromagnet SrCu2(BO3)2 in High Magnetic Fields

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H. Tsujii, R. C. Rotundu, B. Andraka, Y. Takano, ... , Ueda Y.
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We characterize the field-induced magnetic phases of SrCu2(BO3)2, a frustrated spin-1/2 Heisenberg antiferromagnet in the two-dimensional Shastry-Sutherland lattice, using specific heat in magnetic fields up to 33 T. We find that the spin gap persists above the expected critical field Hc = Delta/g*mu_B of 21 T despite the appearance of magnetic moment in the ground state. At the magnetization plateau at 1/8 of the saturation, the Sz = +1 triplets that carry the magnetization ...

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Heat transport by lattice and spin excitations in the spin chain compounds SrCuO_2 and Sr_2CuO_3

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We present the results of measurements of the thermal conductivity of the quasi one-dimensional spin S=1/2 chain compound SrCuO_2 in the temperature range between 0.4 and 300 K along the directions parallel and perpendicular to the chains. An anomalously enhanced thermal conductivity is observed along the chains. The analysis of the present data and a comparison with analogous recent results for Sr_2CuO_3 and other similar materials demonstrates that this behavior is generic ...

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Magnetic Anisotropy of SrCu$_2$(BO$_3$)$_2$ System as Revealed by X-Band ESR

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A. Zorko, D. Arčon, ... , Lappas A.
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X-band ESR measurements on a single crystal of the highly frustrated SrCu$_2$(BO$_3$)$_2$ system are shown to provide an essential inspection of the magnetic anisotropy present in this compound. The very broad absorption lines seem to be consistent with the largest anisotropy term, namely, the antisymmetric Dzyaloshinsky-Moriya (DM) interaction allowed by symmetry. However, the previously well-accepted model of only interdimer interaction is generalized with additional intrad...

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Thermally populated versus field-induced triplon bound states in the Shastry-Sutherland lattice SrCu$_2$(BO$_3$)$_2$

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Dirk Wulferding, Youngsu Choi, Seungyeol Lee, Mikhail A. Prosnikov, Yann Gallais, Peter Lemmens, Chengchao Zhong, ... , Choi Kwang-Yong
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The Shastry-Sutherland compound SrCu$_2$(BO$_3$)$_2$ constituting orthogonally coupled dimers harbors a $S=0$ singlet ground state. The confluence of strong interdimer interaction and frustration engenders a spectrum of low-energy excitations including localized triplons as well as singlet and triplet bound states. Their dynamics are controlled by an external magnetic field and temperature. Here, we employ high-field Raman spectroscopy to map the field and temperature evoluti...

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Far infrared study of the two dimensional dimer spin system SrCu_2(BO_3)_2

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T. Room, U. Nagel, E. Lippmaa, H. Kageyama, ... , Ueda Y.
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Using far-infrared spectroscopy in magnetic fields up to 12T we have studied a two-dimensional dimer spin gap system SrCu_2(BO_3)_2. We found several infrared active modes in the dimerized state (below 10K) in the frequency range from 3 to 100cm^-1. The measured splitting from the ground state to the excited triplet M_S=0 sublevel is Delta_1=24.2cm^-1 and the other two triplet state sublevels in zero magnetic field are 1.4cm^-1 below and above the M_S=0 sublevel. Another mult...

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Correlated decay of triplet excitations in the Shastry-Sutherland compound SrCu$_2$(BO$_3$)$_2$

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M. E. Zayed, Ch. Rüegg, Th. Strässle, U. Stuhr B. Roessli, M. Ay, J. Mesot, P. Link, E. Pomjakushina, M. Stingaciu, ... , Rønnow H. M.
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The temperature dependence of the gapped triplet excitations (triplons) in the 2D Shastry-Sutherland quantum magnet SrCu$_2$(BO$_3$)$_2$ is studied by means of inelastic neutron scattering. The excitation amplitude rapidly decreases as a function of temperature while the integrated spectral weight can be explained by an isolated dimer model up to 10~K. Analyzing this anomalous spectral line-shape in terms of damped harmonic oscillators shows that the observed damping is due t...

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Two band gap field-dependent thermal conductivity of $MgB_2$

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Bai-Mei University of Science and Technology of China, Hefei, PR China Wu, Dong-Sheng Universite de Liege, Belgium, Euroland Yang, Wei-Hua Universite de Liege, Belgium, Euroland Zeng, Shi-Yan Universite de Liege, Belgium, Euroland Li, Bo Universite de Liege, Belgium, Euroland Li, Rong Universite de Liege, Belgium, Euroland Fan, Xian-Hui Universite de Liege, Belgium, Euroland Chen, ... , Ausloos Marcel Universite de Liege, Belgium, Euroland
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The thermal conductivity $\kappa (H,T)$ of the new superconductor $MgB_2$ was studied as a function of the temperature and a magnetic field. No anomaly in the thermal conductivity $\kappa (H,T)$ is observed around the superconducting transition in absence or presence of magnetic fields up to 14 Tesla; upon that field the superconductivity of $MgB_2$ persisted. The thermal conductivity in zero-field shows a $T$-linear increase up to 50K. The thermal conductivity is found to in...

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Evidence for a large magnetic heat current in insulating cuprates

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The in-plane thermal conductivity $k$ of the two-dimensional antiferromagnetic monolayer cuprate Sr$_2$CuO$_2$Cl$_2$ is studied. Analysis of the unusual temperature dependence of $k$ reveals that at low temperatures the heat is carried by phonons, whereas at high temperatures magnetic excitations contribute significantly. Comparison with other insulating layered cuprates suggests that a large magnetic contribution to the thermal conductivity is an intrinsic property of these ...

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NMR evidence for the persistence of spin-superlattice above the 1/8 magnetization plateau in SrCu2(BO3)2

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We present 11B NMR studies of the 2D frustrated dimer spin system SrCu2(BO3)2 in the field range 27-31 T covering the upper phase boundary of the 1/8 magnetization plateau, identified at 28.4 T. Our data provide a clear evidence that above 28.4 T the spin-superlattice of the 1/8 plateau is modified but does not melt even though the magnetization increases. Although this is precisely what is expected for a supersolid phase, the microscopic nature of this new phase is much more...

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Thermal conductivity of YBa2[Cu(1-x)Znx]3O(7-y) single crystals

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The in-plane thermal conductivity K(T) of Zn-doped YBCO single crystals (YBCO:Zn) has been investigated in the temperature range from 5 to 250 K and in magnetic fields up to 30 kOe. The thermal conductivity decreases substantially with increase of the Zn concentration providing reduction in the thermal conductivity peak and its disappearance at a high content of the dopant. At temperatures below 15 K the K(T) dependencies are functionally similar for all the samples. The magn...

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