Pump-probe differencing technique for cavity-enhanced, noise-canceling saturation laser spectroscopy

We study the non-linear interaction of a cold sample of strontium-88 atoms coupled to a single mode of a low finesse optical cavity in the so-called bad cavity limit and investigate the implications for applications to laser stabilization. The atoms are probed on the weak inter-combination line $\lvert 5s^{2} \, ^1 \textrm{S}_0 \rangle \,-\, \lvert 5s5p \, ^3 \textrm{P}_1 \rangle$ at 689 nm in a strongly saturated regime. Our measured observables include the atomic induced ph...

We report a simple method to suppress the light shift in optical pumping systems. This method uses only frequency modulation of a radio frequency or microwave source, which is used to excite an atomic resonance, to simultaneously lock the source frequency to the atomic resonance and lock the pumping light frequency to suppress the light shift. We experimentally validate the method in a vapor-cell atomic clock and verify the results through numerical simulation. This technique...

We have implemented a simple and cost-effective digital system for long-term frequency stabilisation and locking to an arbitrary wavelength of the single-frequency ring CW Ti:Sapphire laser. This system is built around two confocal Fabry-Perot cavities, one of which is used to narrow short-term line width of the laser and the other to improve long-term stability of the laser frequency. The second interferometer is also in the path of the radiation from an external-cavity diod...

We demonstrate that conventional modulated spectroscopy apparatus, used for laser frequency stabilization in many atomic physics laboratories, can be enhanced to provide a wideband lock delivering deep suppression of frequency noise across the acoustic range. Using an acousto-optic modulator driven with an agile oscillator, we show that wideband frequency modulation of the pump laser in modulation transfer spectroscopy produces the unique single lock-point spectrum previously...

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe lasers are independently tunable in frequency, with the probe operating at the single-photon-level. The two-dimensional spectrum measured as the laser frequencies are scanned shows fluorescence, Doppler-broadened absorption dips and sub-Doppler...

We present a novel and simple method of stabilizing the laser phase and frequency by polarization spectroscopy of an atomic vapor. In analogy to the Pound-Drever-Hall method, which uses a cavity as a memory of the laser phase, this method uses atomic coherence (dipole oscillations) as a phase memory of the transmitting laser field. A preliminary experiment using a distributed feedback laser diode and a rubidium vapor cell demonstrates a shot-noise-limited laser linewidth redu...

We present a simple and flexible frequency offset locking scheme developed for high-field imaging of ultra-cold atoms which relies on commercially available RF electronics only. The main new ingredient is the use of the sharp amplitude response of a home-made RF filter to provide an error signal for locking the lasers. We were able to offset lock two independent diode lasers within a capture range of 200 MHz, and with a tuning range of up to 1.4GHz. The beat-note residual flu...

The stabilization of lasers to absolute frequency references is a fundamental requirement in several areas of atomic, molecular and optical physics. A range of techniques are available to produce a suitable reference onto which one can 'lock' the laser, many of which depend on the specific internal structure of the reference or are sensitive to laser intensity noise. We present a novel method using the frequency modulation of an acousto-optic modulator's carrier (drive) signa...

Lasers with high spectral purity are indispensable for optical clocks and coherent manipulation of atomic and molecular qubits for applications such as quantum computing and quantum simulation. Stabilisation of the laser to a reference can provide a narrow linewidth and high spectral purity. However, widely-used diode lasers exhibit fast phase noise that prevents high fidelity qubit manipulation. Here we demonstrate a self-injection locked diode laser system utilizing a mediu...

Comparisons of high-accuracy optical atomic clocks \cite{Ludlow2015} are essential for precision tests of fundamental physics \cite{Safronova2018}, relativistic geodesy \cite{McGrew2018, Grotti2018, Delva2019}, and the anticipated redefinition of the SI second \cite{Riehle2018}. The scientific reach of these applications is restricted by the statistical precision of interspecies comparison measurements. The instability of individual clocks is limited by the finite coherence t...