Pump-probe differencing technique for cavity-enhanced, noise-canceling saturation laser spectroscopy

We present a stabilization technique developed to lock and dynamically tune the resonant frequency of a moderate finesse Fabry-P\'erot (FP) cavity used in precision atom-cavity quantum electrodynamics (QED) experiments. Most experimental setups with active stabilization either operate at one fixed resonant frequency or use transfer cavities to achieve the ability to tune the resonant frequency of the cavity. In this work, we present a simple and cost-effective solution to act...

We demonstrate a new technique for saturated-absorption spectroscopy using co-propagating beams that does not have the problem of crossover resonances. The pump beam is locked to a transition and its absorption signal is monitored while the probe beam is scanned. As the probe comes into resonance with another transition, the pump absorption is reduced and the signal shows a Doppler-free dip. We use this technique to measure hyperfine intervals in the $D_2$ line of $^{85}$Rb w...

We stabilize the idler frequency of a singly-resonant optical parametric oscillator directly to the resonance of a mid-infrared Fabry-P\'erot reference cavity. This is accomplished by the Pound-Drever-Hall locking scheme, controlling either the pump laser or the resonant signal frequency. A residual relative frequency noise power spectral density below 10$^3$ Hz$^2$/Hz is reached, with a Gaussian linewidth of 920 Hz over 100 ms, which demonstrates the potential for reaching s...

We present the accurate measurement of the frequency of the $7S-7P$ laser-trapping transition for three francium isotopes. Our approach is based on an interferometric comparison to deduce the unknown laser frequency from a secondary laser frequency-standard. After careful investigation of systematics, with samples of about 100 atoms the final accuracy reaches 8 MHz, an order of magnitude better than the best previous measurement for $^{210}$Fr, and opens the way to improved t...

We report the frequency stabilization of an erbium-doped fiber distributed-feedback laser using an all-fiber based Michelson interferometer of large arm imbalance. The interferometer uses a 1 km SMF-28 optical fiber spool and an acousto optic modulator allowing heterodyne detection. The frequency noise power spectral density is reduced by more than 40 dB for Fourier frequencies ranging from 1 Hz to 10 kHz, corresponding to a level well below 1 Hz^2/Hz over the whole range. It...

We present a simple, continuous, cavity-enhanced optical absorption measurement technique based on high-bandwidth Pound-Drever-Hall (PDH) sideband locking. The technique provides a resonant amplitude quadrature readout that can be mapped onto the cavity's internal loss rate, and is naturally compatible with weak probe beams. With a proof-of-concept 5-cm-long Fabry-Perot cavity, we measure an absorption sensitivity of $6.6 \times 10^{-11} ~\text{cm}^{-1}/\sqrt{\text{Hz}}$ at 1...

Advances in high-resolution laser spectroscopy have enabled many scientific breakthroughs in physics, chemistry, biology and astronomy. Optical frequency combs have pushed measurement limits with ultrahigh-frequency accuracy and fast-measurement speed while tunable diode laser spectroscopy is used in scenarios that require high power and continuous spectral coverage. Despite these advantages of tunable diode laser spectroscopy, it is challenging to precisely determine the ins...

We present a laser system with a linewidth and long-term frequency stability at the 50 kHz level. It is based on a Ti:Sapphire laser emitting radiation at 882 nm which is referenced to an atomic transition. For this, the length of an evacuated transfer cavity is stabilized to a reference laser at 780 nm locked to the $^{85}$Rb D$_2$-line via modulation transfer spectroscopy. Gapless frequency tuning of the spectroscopy laser is realized using the sideband locking technique to...

The absolute frequencies of the hyperfine components of the R(26) 62-0 transition in molecular iodine at 501.7 nm are measured for the first time with an optical clockwork based on a femtosecond laser frequency comb generator. The set-up is composed of an Ar+ laser locked to a hyperfine component of the R(26) 62-0 transition detected in a continuously pumped low-pressure cell (0.33 Pa). The detected resonances show a linewidth of 45 kHz (half-width at half-maximum). The uncer...

We have developed experimental methods for the generation of chirped laser pulses of controlled frequency evolution in the nanosecond pulse length range for coherent atomic interaction studies. The pulses are sliced from the radiation of a cw external cavity diode laser while its drive current, and consequently its frequency, are sinusoidally modulated. By the proper choice of the modulation parameters, as well as of the timing of pulse slicing, we can produce a wide variety ...